Soil Vapor Monitoring Reflects Dewatering and the Coalgas Isotherm

Ongoing measurements are critical in assessing the effects of Basin-wide water extraction from the Fruitland coalbeds.  As water is produced from coalbeds down-dip from the outcrop, the hydrostatic pressure is reduced most dramatically in the vicinity of each well bore. The influence of coalbed water withdrawal, which is manifested as a decrease in hydrostatic pressure within the various coal seams, would be expected to diminish with increased distance from gas well(s).  Hydrostatic pressure reduction on the coalbeds in turn allows sorbed gas to be desorbed when the pressure is lessened sufficiently.

 

The coal isotherm (Appendix C: Charts 7b) is a graphical representation of the relationship between the release of adsorbed coalgas (in cubic centimeters per gram of coal) and the effects of pressure at a specified temperature.   By consulting this chart, it is possible to predict the equilibrium adsorption/desorption isotherm.  This isotherm depicts the amount of gas anticipated to be released/desorbed from the coal at prevailing conditions of temperature and pressure.

 

Carbon dioxide has a greater affinity for coal than does methane.  Therefore, as reservoir pressure is reduced, methane will be desorbed first.  Thus, early stages of reservoir pressure reduction yield gas with a methane component often in excess of 99 percent by volume.  As reservoir pressure is further reduced, the carbon dioxide component increases.  With each incremental pressure reduction, commensurately more gas will be released, but the carbon dioxide component will account for an increasing portion of the gas mixture. Coalgas production may be limited by economic factors when the carbon dioxide component of the natural gas reaches a threshold concentration at which the cost of carbon dioxide removal is prohibitive.  At current gas prices, this threshold may be breached when the carbon dioxide component of the produced gas stream exceeds 20% by volume.

 

This change in coalgas composition is well illustrated by Appendix C: Chart 12, which illustrates the changes observed in soil gas composition at the Valencia Canyon Gap Collector.  The methane component has decreased from  91% in 1995 to 84% in July1999.  Conversely, the carbon dioxide portion has increased from roughly 9% in 1996 to nearly 16% in July 1999.  In October 1999 soil vapor tube determinations at seven sites surrounding the collector yielded carbon dioxide in concentrations from 15% to 18%.  This same phenomenon may be perpetuated along the entire Fruitland coal outcrop as water saturation of the near-surface coalbeds decrease.  Initial high methane concentrations would be anticipated to decline with a commensurate increase in the carbon dioxide component.  Monitoring for the carbon dioxide component of soil gas was initiated in October/November 1999, revealing carbon dioxide concentrations as high as 36% at one site directly up-canyon from a shallow gas well converted to monitoring status.  Methane decreases may in part reflect the release of greater percentages of carbon dioxide from the coal.  Methylotrophic bacterial oxidation of methane in near-surface environments also produces carbon dioxide (Bennett and Lee, 1996).  One third of the soil vapor tubes showing significant change in methane concentration are decreasing.  The respective gas-to-coal affinity relationship combined with bacterial oxidation effects may explain why some sites along the outcrop exhibit waning (or fluctuating) soil vapor methane (LEL) concentrations.

 

While de-watered Fruitland coal exposures may most readily manifest the influence of low pressures predicted by the coalgas isotherm, similar responses would be anticipated in coalgas wells where the reservoir pressure is reduced at depth.  Indeed, higher carbon dioxide gas content (to 20%) is currently being observed in portions of the basin where reservoir pressures have been reduced the most dramatically.  Northern Basin infill gas wells drilled in 1999 still encounter virgin reservoir pressures and initially produce gas characterized by greater than 99 percent methane and only several tenths of a percent carbon dioxide (Zimmerman, 1999).